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Welcome to TechIMO!!!!
I think it depends on how much money you want to spend. There is about a $40 difference between the 9000 Pro and the Ti4200 with the 9000 Pro being cheaper.
Also, you will most likely only see a difference in benchmarks and not in actual gameplay. Even at 1024x768, the ATI card performs good. And at that those settings, if you can get around 60fps in heavy action, you will not notice the difference if you were getting 100fps.
So what it really boils down to is personal preference. I have always liked ATI cards over Nvidia. ATI is also known for having sharper images than Nvidia, which i like when i am not playing games.
So, it is up to you. I dont think that you will be disapointed with either purchase.
By the way, what is your current hardware setup that you will be adding this card to?
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