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I can be almost sure that this is the cause:
Make sure AA and Anisotropic Filtering are off, I know I've left them on by mistake and wondered why my framerate goes down the tubes.
If CS is running at 99fps, this means you don't have VSync turned on (and you should). Go into your Display properties and turn it on.
I myself have a card almost the same as yours (Ti 4200 at 300/545 aka Ti 4600 core Ti 4400 memory) on an AthlonXP 3200+, and CS runs at a solid 60fps even with 4x AA and 4x Anisotropic Filtering on at 1280x960.
Hope this helps!
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