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Drives are so cheap nowadays its not worth compressing. You may get some files messed up or corrupted. NTFS is a very efficient way to store and if you must, zip the files and save space that way.
Depends what kind of files they are, too. For example, if you have lots of .jpg files you will not save either by zipping or compressinf. These files are compressed already.
If you have lot of .bmp, .doc, .ppt, .xls then you stand to gain a lot of space by zipping and saving on a non-compressed drive.
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